Uniaxial Quadrupole Order in a Magnet With Strong Biquadratic Exchange

Capa

Citar

Texto integral

Acesso aberto Acesso aberto
Acesso é fechado Acesso está concedido
Acesso é fechado Somente assinantes

Resumo

Abstract

It is shown that in a magnet with a sufficiently strong biquadratic exchange interaction (compared to bilinear exchange) and spin S > 1, the temperature transition from a disordered paramagnetic state to the ground ferromagnetic state passes through an intermediate magnetically ordered phase—uniaxial quadrupole ordering. For a magnet with spin S = 3/2, a phase diagram of magnetic states was constructed in the region of large values of the biquadratic exchange and it was studied how the sequence of two phase transitions—“paramagnetic state–quadrupole state” and “quadrupole state–ferromagnetic state”—manifests itself in the temperature behavior of the magnetic heat capacity and the initial magnetic susceptibility.

Sobre autores

E. Kokorina

Institute of Electrophysics, Ural Branch, Russian Academy of Sciences

Autor responsável pela correspondência
Email: kokorina@iep.uran.ru
Russia, 620016, Ekaterinburg

M. Medvedev

Institute of Electrophysics, Ural Branch, Russian Academy of Sciences

Autor responsável pela correspondência
Email: medvedev@iep.uran.ru
Russia, 620016, Ekaterinburg

Bibliografia

  1. Anderson P.W. New approach to the theory of superexchange interactions // Phys. Rev. 1959. V. 115. P. 2−11.
  2. Huang N.L., Orbach R. Biquadratic superexchange // Phys. Rev. Lett. 1964. V. 12. P. 275−277.
  3. Spisak D., Hafner J. Theory of bilinear and biquadratic exchange interactions in iron: bulk and surface // JMMM. 1997. V. 168. P. 257−268.
  4. Kartsev A., Augustin M., Evans R.F.L., Novoselov K.S., Santes E.J.G. Biquadratic exchange interactions in two-dimensional magnets // NPJ: Computational Materials. 2020. 150. 11 p.
  5. Нагаев Э.Л. Магнетики со сложным обменным взаимодействием. М.: Наука. Гл. ред. физ.-мат. лит., 1988. 232 с.
  6. Chen H.H., Levy P.M. Quadrupole phase transitions in magnetic solids // Phys. Rev. Lett. 1971. V. 27. P. 1383.
  7. Chen H.H., Levy P.M. Dipole and quadrupole phase transitions in Spin-1 metals // Phys.Rev. 1973. V. 7. P. 4267−4284.
  8. Кокорина Е.Е., Медведев М.В. Квадрупольное упорядочение и обратный магнитокалорический эффект в магнетике с биквадратичным обменом и спином S = 1 // ФММ. 2022. Т. 123. С. 939−948.
  9. Вальков В.В., Мацулева Г.Н., Овчинников С.Г. Влияние сильного кристаллического поля на спектральные свойства магнетиков с биквадратичным обменом // ФТТ. 1989. Т. 31. Вып. 6. С. 60−67.
  10. Смарт Дж. Эффективное поле в теории магнетизма. М.: Мир, 1968. 272 с.

Arquivos suplementares

Arquivos suplementares
Ação
1. JATS XML
2.

Baixar (42KB)
3.

Baixar (57KB)
4.

Baixar (155KB)